PA-MBE GaN-based optoelectronics on silicon substrates

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Date
2009
Authors
Chuah, Lee Siang
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Abstract
In this project, radio-frequency (RF) nitrogen plasma-assisted molecular beam epitaxy (PA-MBE) technique was used to grow GaN-based layers on Si(111) substrate using high temperature grown AlN as buffer layer. During growth, doping was done using high purity Si and Mg as n- and p-type dopants, respectively. A total of seven techniques were employed to study the properties of the GaN-based films (unintentionally doped n-type GaN, n- and p-doped GaN, unintentionally doped ntype Al0.09Ga0.91N, n-type In0.47Ga0.53N/GaN heterostucture, AlN cap layer/GaN). These were X-ray diffraction (XRD), energy dispersive X-ray analysis (EDX), scanning electron microscopy (SEM), atomic force microscopy (AFM), Hall measurements, photoluminescence (PL) and Raman spectroscopy. The films were evaluated in terms of structural, optical and electrical properties. Since porous GaN-based materials on silicon substrates are a new type of material, the properties are hardly found in the literature. Several different characterization tools have been used to investigate the morphological, structural, and optical properties of porous GaN produced by Pt assisted electroless etching methods. Different features metal contacts on GaN materials have been investigated in this project for the purpose of device fabrication. Nickel was found to have excellent electrical properties and thermal stability at elevated temperatures among the metal contacts on n-type GaN. A Ni/Ag bi-layer ohmic contact on p-GaN has been explored. The specific contact resistivities (SCRs) of this bi-layer scheme were observed to be sensitive to the change of annealing temperatures and durations. Other than that, the study of Schottky contacts based on four different metallization schemes, Ti, Ag, Ti/Ag, and Ag/Ti were performed on p-type GaN, and heat treatment was found able to improve the electrical properties of Schottky contacts generally. Before heat treatment, the Schottky barrier heights (SBHs) of Ti, Ag, Ti/Ag, and Ag/Ti were determined to be 0.58, 0.71, 0.53 and 0.62 eV, respectively. After annealing, the SBHs of Ti, Ti/Ag, and Ag/Ti were found to be 0.67, 0.69 and 0.66 eV, respectively. Following the intensive investigations of material quality and metal contacts, metal-semiconductor-metal (MSM) photodetectors based on porous GaN-based materials were subsequently fabricated and compared to other non-porous-based devices so that the potential of porous GaN-based materials could be fully explored. The study also showed that porous GaN layer was able to enhance the electrical properties of Ni Schottky contacts on GaN in which the SBH and leakage current were improved significantly. Photodetector fabricated from porous GaN layer also showed promising properties in which low dark current and higher photocurrent to dark current ratio were observed. The characteristics of novel GaN-based ultraviolet (UV) Schottky barrier photodiodes with AlN cap layer (50 nm) were presented. Thermal annealing treatment has resulted in improved device characteristics by enhancement of Schottky barrier height, and suppression of dark current of the fabricated Schottky photodiodes. For Schottky diodes annealed at 500 ºC, 600 ºC, and 700 ºC, the dark currents were 3.25 x 10-4, 4.97 x 10-5, and 5.05 x 10-5 A, respectively, under 10 V applied bias. The p-GaN/n-Si heterojunction photodiode was fabricated to observe the photoelectric effects.
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PhD
Keywords
Chemical science , Optoelectronics , Silicon substrates
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